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pH Correction Systems

Acid-base chemistry, titration curves, buffer capacity, reagent demand calculations, and the control strategies that keep pH within setpoint in industrial and wastewater applications.

Acidity, Alkalinity and the Carbonate System

Natural waters resist pH change through the carbonate buffer system. Understanding buffer intensity is essential for sizing reagent doses and predicting control behaviour.

The carbonate buffer system dominates pH behaviour in most natural waters:

Carbonate equilibriaCO₂(aq) + H₂O ⇌ H₂CO₃ ⇌ H⁺ + HCO₃⁻     pK₁ = 6.35
HCO₃⁻ ⇌ H⁺ + CO₃²⁻     pK₂ = 10.33

The buffer intensity β quantifies how much acid or base is needed to change pH by one unit:

Buffer intensityβ = dCb / d(pH) = 2.303 × ([H⁺] + [OH⁻] + CT K₁ [H⁺] / ([H⁺] + K₁)²)

Buffer intensity is at a maximum at pH = pK₁ (6.35) and pH = pK₂ (10.33), and at a minimum near pH 8.3 — the equivalence point of the bicarbonate system. This is why pH 7–8.5 is the hardest region to control: the water has low buffer capacity and a small reagent addition causes a large pH swing.

Worked example: buffer intensity

Water at pH 7.5, alkalinity = 100 mg/L as CaCO₃ (2.0 × 10−3 mol/L), 20°C. Estimate buffer intensity.

[H⁺] = 10−7.5 = 3.16 × 10−8 M    [OH⁻] = 10−6.5 = 3.16 × 10−7 M
K₁ = 10−6.35 = 4.47 × 10−7
β ≈ 2.303 × CT K₁ [H⁺] / ([H⁺] + K₁)² = 2.303 × 2.0×10−3 × 4.47×10−7 × 3.16×10−8 / (4.79×10−7
β ≈ 2.8 × 10−4 eq/L per pH unit
To change pH by 1.0 unit in 1 m³ of water requires 0.28 eq = 14 g CaCO₃ equivalent. This is modest — a small acid/alkali overdose easily overshoots.

Stoichiometric Reagent Sizing

Converting a pH target into a reagent mass requires knowing the water's acid/base demand — typically expressed through acidity, alkalinity or titration to endpoint.

The alkalinity of water is its capacity to neutralise acid. For most waters, alkalinity ≈ [HCO₃⁻] + 2[CO₃²⁻] + [OH⁻] − [H⁺]. In mg/L as CaCO₃:

Acid reagent demand (strong acid)macid (kg/h) = Q (m³/h) × ΔAlk (mg/L as CaCO₃) × Macid / (50,000 × n × P)
Alkali reagent demand (strong base)malkali (kg/h) = Q (m³/h) × ΔAcidity (mg/L as CaCO₃) × Mbase / (50,000 × n × P)

Worked example: sulphuric acid for pH correction

Q = 200 m³/h, initial pH = 9.2, target pH = 7.0. Water alkalinity = 180 mg/L as CaCO₃. At pH 9.2, most alkalinity is HCO₃⁻; to reach pH 7.0 requires neutralising ≈ 70% of bicarbonate = 126 mg/L as CaCO₃. Use 93% H₂SO₄ (M = 98 g/mol, n = 2).

macid = 200 × 126 × 98 / (50,000 × 2 × 0.93) = 2,469,600 / 93,000 = 26.6 kg/h of 93% acid
At 24 h operation = 638 kg/day. Bulk tank (14 days) = 8.9 m³. Specify FRP or HDPE tank with PE liner; 316 SS quill for injection.

Worked example: caustic soda for acidic wastewater

Q = 50 m³/h, pH = 3.5, target pH = 7.0. Acidity titration to pH 7 = 450 mg/L as CaCO₃. Use 50% NaOH (M = 40 g/mol, n = 1, P = 0.50).

mNaOH = 50 × 450 × 40 / (50,000 × 1 × 0.50) = 900,000 / 25,000 = 36 kg/h of 50% NaOH
Pump flow at 50% strength (ρ ≈ 1.53 kg/L, 765 g/L NaOH): q = 36,000 g/h / 765 g/L = 47 L/h. Select 60 L/h motor diaphragm pump, PVDF head, EPDM seals, operating at 78% capacity.

Acid, Base, CO₂ or Lime?

Each reagent has a different reaction speed, buffering effect, cost profile and handling risk. The choice depends on target pH, flow, existing alkalinity and regulatory constraints.

ReagentReactionSpeedBuffer effectBest for
H₂SO₄ (93–98%)2H⁺ + SO₄²⁻InstantAdds sulphate — no bufferLarge flows, pH > 8, industrial
HCl (32%)H⁺ + Cl⁻InstantAdds chloride — no bufferFood-grade, smaller flows
CO₂ (liquid)CO₂ + H₂O → H₂CO₃2–5 minForms HCO₃⁻ — buffers near pH 6.3Potable water, gentle pH reduction
NaOH (25–50%)OH⁻ + H⁺ → H₂OInstantNo buffer; raises Na⁺Industrial effluent, fast correction
Ca(OH)₂ (slurry)OH⁻ + H⁺ → H₂O10–30 minAdds Ca²⁺ + HCO₃⁻ — buffersLarge flows, mining, lowest cost
Na₂CO₃ (soda ash)CO₃²⁻ + H⁺ → HCO₃⁻5–10 minStrong buffer near pH 8.3Moderate pH raise, boiler water

CO₂ dosing for potable water is increasingly popular because it is gentle, food-safe and self-buffering. The stoichiometry is:

CO₂ dose for pH reductionCO₂ + H₂O + HCO₃⁻ → H₂CO₃ + HCO₃⁻ (no net change — the CO₂ converts free OH⁻ or carbonate to bicarbonate)

The practical dose is 5–20 mg/L depending on initial pH and alkalinity. CO₂ is delivered as liquid in pressurised cylinders or bulk tanks, vaporised and injected through a diffuser. No hazardous chemical handling — but the injection system must be gas-tight and the contact tank vented.

pH Control Loop Design

pH is the most nonlinear control variable in water treatment. Fixed-gain PID fails without compensation.

The process gain of a pH loop is the slope of the titration curve at the operating point. Near pH 7 (the equivalence point of most waters), the gain is enormous — a tiny reagent addition causes a large pH swing. At pH 4 or pH 10, the gain is modest.

Design rules for pH control:

Worked example: lime slurry pH raise

Acid mine drainage: Q = 100 m³/h, pH = 3.0, target = 7.5. Titratable acidity = 800 mg/L as CaCO₃. Hydrated lime slurry at 5% w/w (50 g/L Ca(OH)₂).

mCa(OH)2 = 100 × 800 × 74 / (50,000 × 2 × 1.0) = 59.2 kg/h as solid
Slurry flow = 59,200 g/h / 50 g/L = 1,184 L/h of 5% slurry
Select progressive-cavity pump, 1,500 L/h capacity, rubber stator, ceramic-coated rotor. Reaction time ≈ 15 min — size contact/mixing tank for 25 m³ (15 min at 100 m³/h). pH probe after tank; PID with Ti = 5 min, Kp = 0.5 (low gain because of lime's slow response).

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